The tetragonal heavy-fermion superconductor CeRh$_2$As$_2$ ($T_{ \rm c}=0.3$ K) exhibits an exceptionally high critical field of 14 T for $\textbf{ B} \parallel \textbf{ c}$. It undergoes a field-driven first-order phase transition between superconducting (SC) states, potentially transitioning from spin-singlet to spin-triplet superconductivity. To elucidate the underlying pairing mechanism, we probe spin fluctuations in CeRh$_2$As$_2$ using neutron scattering. We find dynamic $(\pi,\pi)$ antiferromagnetic spin correlations with an anisotropic quasi-two-dimensional correlation volume. Our data place an upper limit of 0.31 $\mu_{ \rm B}$ on the staggered magnetization of corresponding N\'{ e}el orders at $T=0.08$ K. Density functional theory (DFT) calculations, treating Ce $4f$ electrons as core states, show that the AFM wave vector connects significant areas of the Fermi surface. Our findings show the dominant excitations in CeRh$_2$As$_2$ for $\hbar\omega< 1.2$~meV are magnetic and indicate superconductivity in CeRh$_2$As$_2$ is mediated by AFM spin fluctuations associated with a proximate quantum critical point.
Categories: cond-mat.str-el cond-mat.supr-con





