We experimentally demonstrate transitions between electronic angular momentum states with a difference in magnetic quantum numbers $\Delta \mathrm{ m_J} = $ 3, 4, and 5 via resonant four- and six-photon stimulated Raman transitions in a single trapped atom. Derivation of the corresponding Rabi frequencies, which are verified experimentally, follows the standard treatment of two-photon transitions including the adiabatic elimination of intermediate states. Finally, we discuss pathways to increase the observed multi-photon transition fidelities to $>99.99\%$, providing a tool for efficient, high-fidelity control of qu\textit{ d}its and single-atom logical qubits.
Categories: quant-ph physics.atom-ph