We provide an explanation of the spin-freezing transition recently observed by Chou et al. (Phys. Rev. Lett. 71, 2323 (1993)) in La_{ 2-x}Sr_x CuO_4 for x <= 0.02. We propose that topological excitations of the 2D Heisenberg quantum antiferromagnet having non-coplanar transverse components have a pair-interaction energy that qualitatively and quantitatively agrees with the observed values of spin-freezing temperature as a function of doping.

Categories: cond-mat

Theory of Coexisting Transverse Spin Freezing and Long-Ranged Antiferromagnetic Order in Lightly Doped La_{2-x}Sr_x CuO_4