A first principles study of La$_{ 2-2x}$Sr$_{ 1+2x}$Mn$_2$O$_7$ compounds for doping levels $0.3\leq x\leq 0.5$ shows that the low energy electronic structure of the majority spin carriers is determined by strong momentum dependent interactions between the Mn $e_g$ $d_{ x^2-y^2}$ and $d_{ 3z^2-r^2}$ orbitals, which in addition to an $x$ dependent Jahn-Teller distortion, differ in the ferromagnetic and antiferromagnetic phases. The Fermi surface exhibits nesting behavior that is reflected by peaks in the static susceptibility, whose positions as a function of momentum have a non-trivial dependence on $x$.
Categories: cond-mat.mtrl-sci